A method of producing a fibrillated liquid crystal polymer powder containing fibrillated liquid crystal polymer particles, comprising, in the following order:
- a grinding step of grinding a biaxially-oriented liquid crystal polymer film to obtain a ground liquid crystal polymer powder having a particle size of 0.1 μm to 300 μm;
- a dispersion preparing step of dispersing the ground liquid crystal polymer powder into a dispersion medium to prepare a dispersion of the ground liquid crystal polymer powder, wherein the dispersion medium has a boiling point not exceeding a melting point of the ground liquid crystal polymer powder;
- a fibrillating step of causing the dispersion of the ground liquid crystal polymer powder to pass through a nozzle under high pressure to crush the ground liquid crystal polymer powder by a wet high-pressure crushing device to obtain the fibrillated liquid crystal polymer powder;
- and
- a dispersion medium removing step of removing the dispersion medium to collect the fibrillated liquid crystal polymer powder.