# US 8,771,452 B2 · Process for producing fiber-reinforced resin material

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- Number: US 8,771,452 B2
- Document ID: US8771452B2
- Status: Granted
- Kind: B2
- Application number: 13/819,150
- Filed: 2010-08-27
- Published: 2013-06-20
- Granted: 2014-07-08
- Earliest claimed: 2010-08-27
- Assignees: Toyota Jidosha Kabushiki Kaisha
- Applicants: Tatsuya Kitagawa
- Inventors: Tatsuya Kitagawa
- Web page: https://patentgrep.com/patent/US8771452B2

## CPC

- B29C 53/24: of plates or sheets
- B29C 65/00: Joining {or sealing} of preformed parts {, e.g. welding of plastics materials}; Apparatus therefor {(general aspects of processes or apparatus for joining preformed parts B29C66/00; using porous material formed by internal pressure generated therein for joining preformed parts B29C44/1228, B29C44/326)}
- B29C 70/504: {using rollers or pressure bands (for corrugating B29C53/22)}
- B32B 3/28: characterised by a layer comprising a deformed thin sheet {, i.e. the layer having its entire thickness deformed out of the plane}, e.g. corrugated, crumpled (B32B29/08 takes precedence)
- B32B 5/12: characterised by the relative arrangement of fibres or filaments of {different layers, e.g. the fibres or filaments being parallel or perpendicular to each other}
- B32B 5/26: another layer {next to it} also being fibrous or filamentary {(relative arrangement of fibres or filaments of different layers B32B5/12)}
- B29C 53/265: {using rolls or endless bands}
- B29C 53/285: {using rolls or endless bands}
- B29C 70/46: using matched moulds, e.g. for deforming sheet moulding compounds [SMC] or prepregs
- B29K 2101/12: Thermoplastic materials
- B32B 2250/20: All layers being fibrous or filamentary
- B32B 2260/023: Two or more layers
- B32B 2260/046: Synthetic resin
- B32B 2262/0269: Aromatic polyamide fibres
- B32B 2262/0276: Polyester fibres
- B32B 2262/101: Glass fibres
- B32B 2262/103: Metal fibres
- B32B 2262/106: Carbon fibres, e.g. graphite fibres
- B32B 2307/52: multi-axially
- B32B 2605/00: Vehicles
- Y10T 156/1016: Transverse corrugating
- Y10T 156/1018: Subsequent to assembly of laminae
- Y10T 156/1039: Surface deformation only of sandwich or lamina [e.g., embossed panels]
- Y10T 156/1044: of parallel stacked sheets only
- B29C: SHAPING OR JOINING OF PLASTICS; SHAPING OF MATERIAL IN A PLASTIC STATE, NOT OTHERWISE PROVIDED FOR; AFTER-TREATMENT OF THE SHAPED PRODUCTS, e.g. REPAIRING (making preforms B29B11/00; making laminated products by combining previously unconnected layers which become one product whose layers will remain together B32B37/00 - B32B41/00)
- B32B: LAYERED PRODUCTS, i.e. PRODUCTS BUILT-UP OF STRATA OF FLAT OR NON-FLAT, e.g. CELLULAR OR HONEYCOMB, FORM
- B29K: INDEXING SCHEME ASSOCIATED WITH SUBCLASSES B29B, B29C OR B29D, RELATING TO MOULDING MATERIALS OR TO MATERIALS FOR {MOULDS, } REINFORCEMENTS, FILLERS OR PREFORMED PARTS, e.g. INSERTS
- Y10T: TECHNICAL SUBJECTS COVERED BY FORMER US CLASSIFICATION

## Abstract

There is provided a process for producing a fiber-reinforced resin material capable of mitigating damage to and defects in reinforcement fibers and of performing lamination with the reinforcement fibers positioned with ease, while at the same time causing them to conform to the shape of the mold with ease at the time of molding. It comprises at least: a step of producing a fiber-reinforced resin sheet (4A) from a reinforcement fiber sheet (2) and a resin sheet (3A) comprising a thermoplastic resin; a step of molding the fiber-reinforced resin sheet (4A) in such a manner as to form a protruding part (4c) on one face (4a) of the fiber-reinforced resin sheet (4A) along one direction and to form a recessed part (4d) along the one direction in another face (4b); a step of laminating the fiber-reinforced resin sheet (5A) while causing at least the protruding part (4c) of the molded fiber-reinforced resin sheet (5A) to engage with a fiber-reinforced resin sheet (5A) that is to be laminated therewith; and a step of molding the laminated fiber-reinforced resin sheets (5A) into the fiber-reinforced resin material while pressurizing and heating them so as to impregnate the reinforcement fibers with the thermoplastic resin.

## Claims

### Claim 1

A process for producing a fiber-reinforced resin material comprising reinforcement fibers and a thermoplastic resin, the process comprising at least:
a step of producing fiber-reinforced resin sheets, each fiber-reinforced resin sheet produced from a reinforcement fiber sheet in which the reinforcement fibers are drawn and aligned in the same direction and a resin sheet comprising the thermoplastic resin;
a step of molding each of the fiber-reinforced resin sheets by heating and pressurizing at least parts of the fiber-reinforced resin sheet corresponding to a protruding part and a recessed part so as to form the protruding part on one face of the fiber-reinforced resin sheet along one direction and to form the recessed part along the one direction in another face located on the opposite side to the protruding part;
a step of laminating the fiber-reinforced resin sheets while causing at least the protruding part of one of the molded fiber-reinforced resin sheets to engage with a fiber-reinforced resin sheet that is to be laminated therewith; and
a step of molding the laminated fiber-reinforced resin sheets into the fiber-reinforced resin material while pressurizing and heating them so as to impregnate the reinforcement fibers with the thermoplastic resin;
wherein, in the step of laminating the fiber-reinforced resin sheets, the fiber-reinforced resin sheets are laminated in such a manner that the protruding parts of the respective fiber-reinforced resin sheets overlap with one another and the recessed parts of the respective fiber-reinforced resin sheets to be laminated with one another overlap with one another;
wherein, in the step of molding the fiber-reinforced resin sheets, the protruding parts protrude in a direction that differs from a direction in which the reinforcement fibers are drawn and aligned;
the step of molding the fiber-reinforced resin sheet comprises:
a step of molding a first fiber-reinforced resin sheet in such a manner as to form the protruding part and the recessed part along a first direction that intersects with a fiber direction in which the reinforcement fibers are drawn and aligned; and
a step of molding a second fiber-reinforced resin sheet in such a manner as to form the protruding part and the recessed part along a second direction that differs from the first direction, and
in the step of laminating the fiber-reinforced resin sheet, the first and second fiberreinforced resin sheets are alternately laminated.

### Claim 2 (depends on 1)

The process according to claim 1, wherein the first direction is a direction that is orthogonal to the fiber direction, and the second direction is a direction along the fiber direction.

### Claim 3 (depends on 1)

The process according to claim 1, wherein the first direction is a direction that intersects with the fiber direction at a predetermined angle, and the second direction is a direction that is along the fiber direction or orthogonal to the fiber direction.

### Claim 4 (depends on 1)

The process according to claim 1, wherein, in the step of molding the fiber-reinforced resin sheet, using a pair of heating rollers in which at least a protruding ridge part is formed on an outer roller circumferential surface of one of the heating rollers and a recessed groove part corresponding to the shape of the protruding ridge part is formed in an outer roller circumferential surface of the other heating roller, the protruding part and the recessed part are molded by performing pressurizing and heating while sandwiching the fiber-reinforced resin sheet between the protruding ridge part and the recessed groove part between the pair of heating rollers.

### Claim 5 (depends on 1)

The process according to claim 1, wherein, in the step of molding the fiberreinforced resin sheets, the protruding part and the recessed part are molded in such a manner that the fiber-reinforced resin sheet becomes a corrugated sheet having a given cycle.

### Claim 6 (depends on 1)

The process according to claim 1, wherein, in the step of producing the fiberreinforced resin sheets, a reinforcement fiber sheet in which a reinforcement fiber bundle is spread is used as the reinforcement fibers.

### Claim 7

A process for producing a fiber-reinforced resin material comprising reinforcement fibers and a thermoplastic resin, the process comprising at least:
a step of producing fiber-reinforced resin sheets, each fiber-reinforced resin sheet produced from a reinforcement fiber sheet in which the reinforcement fibers are drawn and aligned in the same direction and a resin sheet comprising the thermoplastic resin;
a step of molding each of the fiber-reinforced resin sheets by heating and pressurizing at least parts of the fiber-reinforced resin sheet corresponding to a protruding part and a recessed part so as to form the protruding part on one face of the fiber-reinforced resin sheet along one direction and to form the recessed part along the one direction in another face located on the opposite side to the protruding part;
a step of laminating the fiber-reinforced resin sheets while causing at least the protruding part of one of the molded fiber-reinforced resin sheets to engage with a fiber-reinforced resin sheet that is to be laminated therewith; and
a step of molding the laminated fiber-reinforced resin sheets into the fiber-reinforced resin material while pressurizing and heating them so as to impregnate the reinforcement fibers with the thermoplastic resin;
in the step of producing the fiber-reinforced resin sheet, a sheet of resin fibers comprising a thermoplastic resin is used as the thermoplastic resin sheet, and the fiber-reinforced resin sheet is produced in such a manner that the resin fibers are disposed by being drawn and aligned along the same direction as the fiber direction in which the reinforcement fibers are drawn and aligned,
in the step of molding the fiber-reinforced resin sheet, the fiber-reinforced resin sheet is molded by melting the thermoplastic resin only of parts corresponding to the protruding part and the recessed part in such a manner that the protruding part and the recessed part intersect with at least the fiber direction, and
in the step of laminating the fiber-reinforced resin sheet, the fiber-reinforced resin sheet is laminated in such a manner that the protruding part of the fiber-reinforced resin sheet is inserted between fibers including the reinforcement fibers and the resin fibers of the fiber-reinforced resin sheet that is to be laminated therewith.

### Claim 8 (depends on 7)

The process according to claim 7, wherein, in the step of producing the fiber-reinforced resin sheets, a reinforcement fiber sheet in which a reinforcement fiber bundle is spread is used as the reinforcement fibers.

### Claim 9 (depends on 7)

The process according to claim 7, wherein, in the step of molding the fiber-reinforced resin sheet, using a pair of heating rollers in which at least a protruding ridge part is formed on an outer roller circumferential surface of one of the heating rollers and a recessed groove part corresponding to the shape of the protruding ridge part is formed in an outer roller circumferential surface of the other heating roller, the protruding part and the recessed part are molded by performing pressurizing and heating while sandwiching the fiber-reinforced resin sheet between the protruding ridge part and the recessed groove part between the pair of heating rollers.

### Claim 10 (depends on 7)

The process according to claim 7, wherein, in the step of laminating the fiber-reinforced resin sheets, the fiber-reinforced resin sheets are laminated in such a manner that the protruding parts of the respective fiber-reinforced resin sheets overlap with one another, and the recessed parts of the respective fiber-reinforced resin sheets to be laminated with one another overlap with one another.

### Claim 11 (depends on 10)

The process according to claim 10, wherein, in the step of molding the fiber-reinforced resin sheets, the protruding parts protrude in a direction that differs from a direction in which the reinforcement fibers are drawn and aligned.

### Claim 12 (depends on 7)

The process according to claim 7, wherein, in the step of molding the fiber-reinforced resin sheets, the protruding part and the recessed part are molded in such a manner that the fiber-reinforced resin sheet becomes a corrugated sheet having a given cycle.
