In a nuclear reactor comprising a core of nuclear fuel elements, a downcomer annulus between a pressure vessel and said core, means for feeding feedwater into said pressure vessel, means for forcing said feedwater to flow through said core to cool said fuel elements, and means for separating steam and water phases in the mixture exiting said core, said water phase flowing from said steam/water separating means to said downcomer annulus, the improvement wherein catalytic ammonia conversion means are arranged upstream of said steam/water separating means and downstream of said fuel elements, said catalytic ammonia conversion means comprising catalytic material arranged in an open structure disposed so that substantially all of the water/steam mixture entering said steam/water separating means flows therethrough, and said catalytic material having a surface area-to-volume ratio sufficiently high enough to catalyze the conversion of ammonia and/or NO in said water/steam mixture into nitrite or nitrate.