A method of manufacturing an organic substrate used for printed circuits, which comprises the steps of forming through-holes in a porous raw material provided with free tackness films and having compressive shrinkage comprising a composite material of a non-woven fabric and a thermosetting resin, filling electro-conductive paste into said through-holes, and also increasing composition ratio of the electro-conductive material with respect to a binder in the electro-conductive paste, separating the free tackness films from said porous raw material filled with the electro-conductive paste in the through-holes thereof, applying metal foils onto the surface of said porous raw material from which said free tackness films have been separated, and then compressing said porous raw material applied with said metal foils through heating and pressurization so as to make more compact, the electro-conductive material in said electro-conductive paste.