# US 5,326,650 A · Solid oxide fuel electrodes and process for producing

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- Number: US 5,326,650 A
- Document ID: US5326650A
- Status: Granted
- Kind: A
- Application number: 08/044,108
- Filed: 1993-04-09
- Granted: 1994-07-05
- Earliest claimed: 1992-03-26
- Assignees: NGK Insulators, Ltd.
- Inventors: Yoshihiko Ishida
- Web page: https://patentgrep.com/patent/US5326650A

## CPC

- H01M 8/0215: Glass; Ceramic materials
- H01M 8/0228: in the form of layered or coated products
- H01M 8/0247: characterised by the form (characterised by a channel configuration H01M8/0258)
- H01M 8/1213: characterised by the electrode/electrolyte combination or the supporting material
- H01M 8/2432: Grouping of unit cells of planar configuration
- H01M 8/2465: Details of groupings of fuel cells
- Y02E 60/50: Fuel cells
- Y02P 70/50: Manufacturing or production processes characterised by the final manufactured product
- H01M: PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- Y02E: REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
- Y02P: CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS

## Abstract

A solid oxide fuel cell is disclosed, which includes flat plate-shaped solid oxide fuel cell elements. The solid oxide fuel cell element includes an ion-conductive ceramic plate, and an air electrode and a fuel electrode formed on opposite surfaces of the ion-conductive ceramic plate, respectively, wherein conductive strips which have less resistance than the electrode are continuously formed on a surface of at least one of the air electrode and the fuel electrode. A solid oxide fuel cell is also disclosed, which includes a separator plate made of a material having oxidation resistance, reduction resistance and electron conductivity, an air electrode spacer made of a material having oxidation resistance and electron conductivity, the above flat plate-shaped solid oxide fuel cell element, and a fuel electrode spacer made of a material having reduction resistance and electron conductivity, wherein the separator plate, the air electrode spacer, the flat plate-shaped solid oxide fuel cell element and the fuel electrode spacer are successively laminated in this order. An oxidizing gas chamber is defined by the separator plate, the air electrode spacer and the element, and a fuel gas chamber is defined by the separator plate, the fuel electrode spacer and the element. A process is also disclosed for producing such a solid oxide fuel cell element.

## Claims

### Claim 1

A solid oxide fuel cell comprising a separator plate made of a material having oxidation resistance, reduction resistance and electron conductivity, an air electrode spacer made of a material having oxidation resistance and electron conductivity, a flat plate-shaped solid oxide fuel cell element, a fuel electrode spacer made of a material having reduction resistance and electron conductivity and another spacer plate made of a material having oxidation resistance, reduction resistance and electron conductivity, said separator plate, said air electrode spacer, said flat plate-shaped solid oxide fuel cell element, said fuel electrode spacer and said another spacer plate being successively laminated in this order,
said solid oxide fuel cell element comprising an ion-conductive ceramic plate, and an air electrode and a fuel electrode formed on opposite surfaces of said ion-conductive ceramic plate, respectively, wherein conductive strips which have less resistance than said electrode are formed in a continuous pattern on a surface of at least one of said air electrode and said fuel electrode,
wherein an oxidizing gas chamber is defined by said separator plate, said air electrode spacer and said fuel cell element, and a fuel gas chamber is defined by said another separator plate, said fuel electrode spacer and said fuel cell element.

### Claim 2 (depends on 1)

The solid oxide fuel cell as set forth in claim 1, wherein said separator plates are square flat plates whose four sides are formed with rectangular projections, respectively, each of said air electrode spacer and said fuel electrode spacer has a substantially U-shaped form including a pair of aligned projections outwardly extending from ends of legs of the U-shaped form and a rectangular projection outwardly extending from a bottom of the U-shaped form, and said flat plate-shaped solid oxide fuel cell element is a square flat plate whose four sides are formed with rectangular projections to conform with the projections of the separator plates and the spacers.

### Claim 3 (depends on 1)

The solid oxide fuel cell as set forth in claim 1, wherein said separator plates are substantially square flat plates each formed with an oxidizing gas opening and a fuel gas opening, respectively, said air electrode spacer is a substantially square flat late formed with a substantially square punched portion convexed at its corner where a fuel gas opening is formed, said flat plate-shaped solid oxide fuel cell element is a square flat plate formed with an oxidizing gas opening and a fuel gas opening, and said fuel electrode spacer is substantially a square flat plate formed with a substantially square punched portion convexed at its corner where an oxidizing gas opening is formed, said oxidizing gas opening and said fuel gas opening of the fuel element being in conformity with said oxidizing gas opening of the air electrode spacer and said fuel gas opening of the fuel electrode spacer, respectively.