In a process for controlling oxides of nitrogen in exhaust gases from combustion equipment by decomposing the oxides with oxygen and ammonia at temperatures from 700 .degree. to 1300.degree. C., the improvement which comprises arranging a catalyst assembly downstream of the contact point between the exhaust gas and ammonia, with the catalytic surfaces of the component units of the assembly substantially in parallel to the direction of gas flow, in a region where the temperature of the gas after the decomposing treatment is from 300.degree. and 500.degree. C., so that the said gas after said decomposing treatment may pass through said catalyst assembly, and introducing an additional supply of ammonia, in an amount of from 0.5 to 1.5 times equivalent (in molar ratio) to the amount of nitrogen oxides in moles in said gas, into the space immediately upstream of said catalyst assembly, thereby to accelerate the decomposition of said oxides in said gas to harmless substances.