# US 11,112,355 B2 · Narrowband, acoustically mediated spintronic terahertz emitter

> Agents: this data is available as JSON from the patentgrep API and MCP server — see https://patentgrep.com/llms.txt

- Number: US 11,112,355 B2
- Document ID: US11112355B2
- Status: Granted
- Kind: B2
- Application number: 16/727,308
- Filed: 2019-12-26
- Published: 2021-07-01
- Granted: 2021-09-07
- Earliest claimed: 2019-12-26
- Assignees: Wisconsin Alumni Research Foundation
- Applicants: Wisconsin Alumni Research Foundation
- Inventors: Jiamian Hu; Shihao Zhuang
- Web page: https://patentgrep.com/patent/US11112355B2

## CPC

- G01N 21/3586: by Terahertz time domain spectroscopy [THz-TDS]
- G02F 2/02: Frequency-changing of light, e.g. by quantum counters
- G01N 2201/06113: Coherent sources; lasers
- G02F 2203/13: involving THZ radiation
- H01S 3/0092: {Nonlinear frequency conversion, e.g. second harmonic generation [SHG] or sum- or difference-frequency generation outside the laser cavity (nonlinear frequency conversion per se G02F1/35)}
- G01N: INVESTIGATING OR ANALYSING MATERIALS BY DETERMINING THEIR CHEMICAL OR PHYSICAL PROPERTIES (measuring or testing apparatus or processes other than immunoassay, involving enzymes or microorganisms C12M, C12Q)
- G02F: OPTICAL DEVICES OR ARRANGEMENTS FOR THE CONTROL OF LIGHT BY MODIFICATION OF THE OPTICAL PROPERTIES OF THE MEDIA OF THE ELEMENTS INVOLVED THEREIN; NON-LINEAR OPTICS; FREQUENCY-CHANGING OF LIGHT; OPTICAL LOGIC ELEMENTS; OPTICAL ANALOGUE/DIGITAL CONVERTERS
- H01S: DEVICES USING THE PROCESS OF LIGHT AMPLIFICATION BY STIMULATED EMISSION OF RADIATION [LASER] TO AMPLIFY OR GENERATE LIGHT; DEVICES USING STIMULATED EMISSION OF ELECTROMAGNETIC RADIATION IN WAVE RANGES OTHER THAN OPTICAL

## Abstract

Acoustically mediated spintronic THz emitters in which sound waves, rather than direct laser pulses, give rise to a spin current in a magnetic material via magnetoelastic coupling are provided. The THz emitters include a metal layer that acts as a light-to-acoustic transducer. Also provided are THz time-domain spectrometers (THz-TDSs) that incorporate the THz emitters.

## Claims

### Claim 1

A heterostructure comprising:
a transducer layer having a first surface and consisting of a metal selected from the group consisting of aluminum, iron, platinum, gold, cobalt, and nickel;
a thermal insulation layer adjacent to a second surface of the transducer layer opposite the first surface;
a magnetic layer comprising a ferromagnetic or ferrimagnetic material in contact with a surface of the thermal insulation layer opposite the transducer layer, such that the thermal insulation layer is disposed between the transducer layer and the magnetic layer; and
a heavy metal layer comprising a heavy metal adjacent to a surface of the magnetic layer opposite the thermal insulation layer, such that the magnetic layer is disposed between the thermal insulation layer and the heavy metal layer.

### Claim 2 (depends on 1)

The heterostructure of claim 1, wherein the thermal insulation layer is a layer of magnesium oxide, the magnetic layer is a layer of FeGa, and the heavy metal layer is a layer of platinum.

### Claim 3

A heterostructure comprising:
a transducer layer having a first surface and consisting of a metal selected from the group consisting of aluminum, iron, platinum, gold, cobalt, and nickel;
a thermal insulation layer adjacent to a second surface of the transducer layer opposite the first surface;
a magnetic layer comprising a ferromagnetic or ferrimagnetic material adjacent to a surface of the thermal insulation layer opposite the transducer layer, such that the thermal insulation layer is disposed between the transducer layer and the magnetic layer; and
a heavy metal layer comprising a heavy metal adjacent to a surface of the magnetic layer opposite the thermal insulation layer, such that the magnetic layer is disposed between the thermal insulation layer and the heavy metal layer, wherein the thermal insulation layer has a thickness in the range from 400 nm to 500 μm, the transducer layer has a thickness in the range from 10 nm to 25 nm, and the magnetic layer has a thickness of at least 50 nm.

### Claim 4 (depends on 3)

The heterostructure of claim 3, wherein the thermal insulation layer is a single-crystalline layer and the magnetic layer is a single-crystalline layer.

### Claim 5 (depends on 4)

The heterostructure of claim 4, wherein the thermal insulation layer is a layer of magnesium oxide, the transducer layer is a layer of aluminum or a layer of iron, the magnetic material is FeGa, and the heavy metal is platinum.

### Claim 6 (depends on 3)

The heterostructure of claim 3, wherein the magnetic layer is a polycrystalline layer or an amorphous layer.

### Claim 7 (depends on 6)

The heterostructure of claim 6, wherein the thermal insulation layer is a layer of magnesium oxide, the transducer layer is a layer of aluminum or a layer of iron, the magnetic material is FeGa, and the heavy metal is platinum.

### Claim 8

A terahertz radiation source comprising:
(a) a heterostructure comprising:
(i) a transducer layer having a light receiving surface and consisting of a metal selected from the group consisting of aluminum, iron, platinum, gold, cobalt, and nickel;
(ii) a thermal insulation layer adjacent to a surface of the transducer layer opposite the light receiving surface;
(iii) a magnetic layer comprising a ferromagnetic or ferrimagnetic material in contact with a surface of the thermal insulation layer opposite the transducer layer, such that the thermal insulation layer is disposed between the transducer layer and the magnetic layer; and
(iv) a heavy metal layer comprising a heavy metal adjacent to a surface of the magnetic layer opposite the thermal insulation layer, such that the magnetic layer is disposed between the thermal insulation layer and the heavy metal layer; and
(b) a femtosecond pulse laser positioned to direct femtosecond laser pulses onto the light receiving surface of the transducer layer.

### Claim 9 (depends on 8)

The terahertz radiation source of claim 8, wherein the thermal insulation layer is a layer of magnesium oxide, the magnetic layer is a layer of FeGa, and the heavy metal layer is a layer of platinum.

### Claim 10

A method of generating THz radiation using a terahertz radiation source comprising:
(a) a heterostructure comprising:
(i) a transducer layer having a light receiving surface and consisting of a metal selected from the group consisting of aluminum, iron, platinum, gold, cobalt, and nickel;
(ii) a thermal insulation layer adjacent to a surface of the transducer layer opposite the light receiving surface;
(iii) a magnetic layer comprising a ferromagnetic or ferrimagnetic material adjacent to a surface of the thermal insulation layer opposite the transducer layer, such that the thermal insulation layer is disposed between the transducer layer and the magnetic layer; and
(iv) a heavy metal layer comprising a heavy metal adjacent to a surface of the magnetic layer opposite the thermal insulation layer, such that the magnetic layer is disposed between the thermal insulation layer and the heavy metal layer; and
(b) a femtosecond pulse laser positioned to direct femtosecond laser pulses onto the light receiving surface of the transducer layer, the method comprising:
irradiating the light receiving surface of the transducer layer with femtosecond laser pulses from the femtosecond pulse laser to generate acoustic pulses that traverse the thermal insulation layer and are injected into the magnetic layer to generate a spin current in the magnetic layer, wherein the spin current is converted into a charge current in the heavy metal layer that gives rise to THz radiation emission from the heavy metal layer.

### Claim 11 (depends on 10)

The method of claim 10, wherein the thermal insulation layer has a thickness in the range from 400 nm to 500 μm, the transducer layer has a thickness in the range from 10 nm to 25 nm, and the magnetic layer has a thickness of at least 50 nm.

### Claim 12 (depends on 10)

The method of claim 10, wherein the thermal insulation layer is a layer of magnesium oxide, the magnetic layer is a layer of FeGa, and the heavy metal layer is a layer of platinum.

### Claim 13

A terahertz time-domain spectrometer comprising:
a femtosecond pulse laser that emits a pulsed femtosecond laser beam;
a beam splitter in a path of the pulse femtosecond laser beam, wherein the beam splitter splits the pulsed femtosecond laser beam into a pump beam and a probe beam;
the heterostructure comprising:
a transducer layer having a light receiving surface and consisting of a metal selected from the group consisting of aluminum, iron, platinum, gold, cobalt, and nickel;
a thermal insulation layer adjacent to a surface of the transducer layer opposite the light receiving surface;
a magnetic layer comprising a ferromagnetic or ferrimagnetic material in contact with a surface of the thermal insulation layer opposite the transducer layer, such that the thermal insulation layer is disposed between the transducer layer and the magnetic layer; and
a heavy metal layer comprising a heavy metal adjacent to a surface of the magnetic layer opposite the thermal insulation layer, such that the magnetic layer is disposed between the thermal insulation layer and the heavy metal layer, wherein the heterostructure is configured in a path of the pump beam such that the pump beam irradiates the transducer layer;
a terahertz detector, configured to detect a terahertz pulse output signal emitted from the heterostructure; and
a delay line assembly configured in the path of the probe beam to create an adjustable time delay in the probe beam and to direct the probe beam onto the terahertz detector.

### Claim 14 (depends on 13)

The terahertz time-domain spectrometer of claim 13, wherein the thermal insulation layer has a thickness in the range from 400 nm to 500 μm, the transducer layer has a thickness in the range from 10 nm to 25 nm, and the magnetic layer has a thickness of at least 50 nm.

### Claim 15 (depends on 13)

The terahertz time-domain spectrometer of claim 13, wherein the thermal insulation layer is a layer of magnesium oxide, the magnetic layer is a layer of FeGa, and the heavy metal layer is a layer of platinum.

### Claim 16

A terahertz radiation source comprising:
(a) a heterostructure comprising:
(i) a transducer layer having a light receiving surface and consisting of a metal selected from the group consisting of aluminum, iron, platinum, gold, cobalt, and nickel;
(ii) a thermal insulation layer adjacent to a surface of the transducer layer opposite the light receiving surface;
(iii) a magnetic layer comprising a ferromagnetic or ferrimagnetic material adjacent to a surface of the thermal insulation layer opposite the transducer layer, such that the thermal insulation layer is disposed between the transducer layer and the magnetic layer; and
(iv) a heavy metal layer comprising a heavy metal adjacent to a surface of the magnetic layer opposite the thermal insulation layer, such that the magnetic layer is disposed between the thermal insulation layer and the heavy metal layer; and
(b) a femtosecond pulse laser positioned to direct femtosecond laser pulses onto the light receiving surface of the transducer layer, wherein the thermal insulation layer has a thickness in the range from 400 nm to 500 μm, the transducer layer has a thickness in the range from 10 nm to 25 nm, and the magnetic layer has a thickness of at least 50 nm.