An admixture composition, for improving the hydrophobicity of a cementitious material that comprises a cement mixture with hydrated cement particles dispersed therein, which comprises solid polymer particles that have a surface coating comprising a blend of a surfactant and a hydrophobic agent which is selected from the group consisting of waste lubricant oil, spent motor oil, base oil, ester of fatty acids, vegetable oil, and mixtures thereof, wherein the solid polymer particles adhere to exterior surfaces of the hydrated cement particles, and fine particles that are selected from the group consisting of activated carbon, silica fume, spent catalyst, and mixtures thereof.